The 51-year-old professional quizzer – better known as The Beast – was left frustrated after the four-person team reigned victorious.
He was seen hitting his fist as he sat at his table after he found out he was out of time and had lost with just three questions left to answer.
Mark told them: “You put me under pressure,” as he congratulated them for beating him. The final round saw him losing after getting six questions wrong and four successful push backs by the team.
He also felt the heat and leapt in prematurely before quiz master Bradley Walsh finished asking a question, resulting in Mark giving the wrong answer and the team pushing him back one step.
It was clear that The Beast was struggling after he failed to eliminated any of the four players from The Chase in the head-to-head rounds.
All of the team played it safe as well and stuck to their cash builder money rather than taking the tempting higher offer and a step closer to The Chaser.
Even civil servant Mahtab from Bradford, who secured an impressive £9,000 in the first round, stuck to his guns and made it back to the team, even though he could have gone for the higher offer several times.
“What’s wrong with these people?” Mark exclaimed to Bradley, 56, after another person turned down the higher offer.
This is not the first time The Beast has lost his temper on The Chase, he previously punched a wall and stormed off after he lost out to a different team.
He recently revealed that he had actually won the game before the adjudicators had decided that he had made a mistake in his answer.
The Beast told Express.co.uk: “Because it’s been edited down […] they actually gave me the answer originally. I’d gone on with a couple of questions and then they went, ‘Hang on a minute!’.
“They went back and looked at it all again on slow motion replay and picked up I’d added an ’s’ and then they went, ‘no, no, you can’t have it’.
“That went wrong. I’d won the game to I’ve lost it. Now any sportsman would tell you, when that happens, it hurts.”
The Chase airs weekdays on ITV at 5pm.